基于气液多相反应过程强化的CO2捕集研究进展Research progress on CO2 capture based on intensification of gas-liquid multiphase reaction processes
张亚栋,张伟,詹水清,王家乐,王军锋
摘要(Abstract):
高效碳捕集技术的开发是实现“双碳”目标的关键路径。化学吸收法因传质效率高、反应速率快和工艺成熟等优点,已成为燃烧后碳捕集的重要技术方案。近年来,该方法在吸收剂开发、气泡行为调控、传质机制解析及反应器结构设计等方面取得了显著进展,但在能耗控制、界面稳定性与过程强化路径等方面仍存在诸多挑战。本文重点综述了典型吸收剂体系及其协同机制、气泡分散特性与多相界面传质行为、反应器结构优化方法以及关键操作参数对系统性能的影响,评估了电场、磁场等外加物理场的协同调控潜力。从多尺度建模、相分散特性强化与功能材料设计等角度提出了未来的研究方向,以期为构建高效、低能耗、环境友好的碳捕集系统提供理论依据与技术参考。
关键词(KeyWords): 鼓泡反应器;二氧化碳捕集;气泡;化学吸收剂;传质效率;多相反应
基金项目(Foundation): 国家自然科学基金项目(52206201,52476154)
作者(Author): 张亚栋,张伟,詹水清,王家乐,王军锋
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