轻重相交替进料筛板萃取塔中的传质性能研究Research on Mass Transfer in a Perforated-Plate Extraction Column with Alternating Feeding of Light and Heavy Phases
王喆,窦梅,南碎飞
摘要(Abstract):
针对间歇操作萃取工艺生产能力低,而逆流连续操作萃取工艺返混严重等问题,研究提出了轻重相交替进料操作的萃取工艺,并对轻重相交替进料筛板萃取塔中的传质性能进行了研究。以煤油-苯甲酸-水为萃取体系,采用单个液滴的传质模型来计算萃取塔的分散相总传质系数,并研究了分散相流速、连续相流速、液滴上升速度以及塔板间距对分散相总传质系数的影响。实验得到分散相总传质系数Kod的数值在3.49?10?5~5.47?10?5 m?s?1,总分散相存留分数在1.63%~4.37%。结果表明轻重相交替进料筛板萃取塔的分散相总传质数高于Kühni搅拌萃取塔、脉冲萃取塔和振动挡板塔,并且流量变化对Kod的影响小,返混效应弱,总分散相存留分数小,不易液泛。
关键词(KeyWords): 轻重相交替进料;筛板萃取塔;返混;分散相存留;传质系数
基金项目(Foundation):
作者(Author): 王喆,窦梅,南碎飞
参考文献(References):
- [1]FEI Wei-yang(费维扬).Progresses of study and application on extraction columns(萃取塔设备研究和应用的若干新进展)[J].Journal of Chemical Industry and Engineering(China)(化工学报),2013,64(1):44-51.
- [2]Lade V G,Rathod V K,Bhattacharyya S,et al.Comparison of normal phase operation and phase reversal studies in a pulsed sieve plate extraction column[J].Chemical Engineering Research&Design,2013,91(6):1133-1144.
- [3]Bahmanyar H,Nazari L,Sadr A.Prediction of effective diffusivity and using of it in designing pulsed sieve plate extraction columns[J].Chemical Engineering&Processing,2008,47(1):57-65.
- [4]ZHAO Qiu-yue(赵秋月),ZHANG Ting-an(张廷安),LIU Yan(刘燕),et al.Effect of stirring on liquid-liquid separation in modified mixer-settlers(高效澄清萃取槽内搅拌对液液分离特性的影响)[J].Journal of Chemical Engineering of Chinese Universities(高校化学工程学报),2014,28(3):530-534.
- [5]Hlawitschka M W,Bart H J.Determination of local velocity,energy dissipation and phase fraction with LIF-and PIV-measurement in a Kühni miniplant extraction column[J].Chemical Engineering Science,2012,69(1):138-145.
- [6]Stella A,Mensforth K H,Bowser T,et al.Mass transfer performance in karr reciprocating plate extraction columns[J].Industrial&Engineering Chemistry Research,2008,47(11):3996-4007.
- [7]Noh S.H,Baird M H I.Mass transfer and pressure drop in a cocurrent reciprocating plate extraction column[J].AICh E Journal,1984,30(1):120-127.
- [8]Shen Z J,Rama Rao N V,Baird M H I.Mass transfer in a reciprocating plate extraction column-effects of mass transfer direction and plate material[J].Canadian Journal of Chemical Engineering,1985,63(1):29-36.
- [9]Camurdan M C,Baird M H I,Taylor P A.Steady state hydrodynamics and mass transfer characteristics of a karr extraction column[J].Canadian Journal of Chemical Engineering,1989,67(4):554-559.
- [10]Stella A,Pratt H R C,Mensforth K H,et al.Backmixing in karr reciprocating-plate extraction columns[J].Industrial&Engineering Chemistry Research,2006,45(19):6555-6562.
- [11]Gomes L N,Guimar?es M L,Regueiras P F R,et al.Simulated and experimental dispersed-phase breakage and coalescence behavior in a kühni liquid-liquid extraction column-steady state[J].Industrial&Engineering Chemistry Research,2006,45(11):3955-3968.
- [12]Hemmati A,Torab-Mostaedi M,Asadollahzadeh M.Mass transfer coefficients in a Kühni extraction column[J].Chemical Engineering Research&Design,2015,93:747-754.
- [13]Rincón-Rubio L M,Kumar A,Hartland S.Characterization of flooding in a Wirz extraction column[J].The Canadian Journal of Chemical Engineering,1993,71(6):844-851.
- [14]Takahashi K,Abdel-Tawab A S,Nii S,et al.Extraction of rare earth metals with a multistage mixer-settler extraction column[J].Chemical Engineering Science,2002,57(3):469-478.
- [15]Torab-Mostaedi M,Safdari J,Moosavian M A,et al.Stage efficiency of Hanson mixer-settler extraction column[J].Chemical Engineering&Processing,2009,48(1):224-228.
- [16]Takahashi K,Nakashima H,Nii S,et al.Maximum throughput in multistage mixer-settler extraction column[J].Chemical Engineering,1993,19(3):440-445.
- [17]Bahmanyar A,Khoobi N,Mozdianfard M R,et al.The influence of nanoparticles on hydrodynamic characteristics and mass transfer performance in a pulsed liquid–liquid extraction column[J].Chemical Engineering&Processing Process Intensification,2011,50(11-12):1198-1206.
- [18]Amanabadi M,Bahmanyar H.Prediction of effective diffusion coefficient in rotating disc columns and application in design[J].Chinese Journal of Chemical Engineering,2009,17(3):366-372.
- [19]Torab-Mostaedi M,Safdari J.Prediction of mass transfer coefficients in a pulsed packed extraction column using effective diffusivity[J].Brazilian Journal of Chemical Engineering,2009,26(4):685-694.
- [20]Napeida M,Asl A H,Safdari J,et al.Holdup and characteristic velocity in a Hanson mixer–settler extraction column[J].Chemical Engineering Research&Design,2010,88(5):703-711.